We report imperceptibly micro-wrinkled organic light-emitting diodes (OLEDs) to define distortion-free pixel by in-situ deposition on two-dimensionally pre-stretched polydimethylsiloxane (PDMS) substrate. The developed fabrication process includes surface engineering for a low-temperature solution process. After releasing the pre-strain, a micro-wrinkled structure facilitates to maintain the clear shape of the pixel with the wrinkle period under 20 µm that is unrecognizable to the human eyes, whereas wrinkles of hundreds of µm are formed when using plastic films. The micro-wrinkled OLEDs show a luminance over 8,000 cd/m2, a maximum current efficiency of 7 cd/A and can endure two-dimensional 20% strain. Our in-situ fabrication method can become a new framework for stretchable OLEDs with simple and low-cost fabrication with improved visibility.
We report a facile fabrication method of curved mirror with 3D printed plastic mold. Polylactic acid (PLA) is used as material for plastic mold. Polydimethylsiloxane (PDMS) replica is obtained from PLA mold, followed by planarization with spin-coating of additional PDMS. After ultraviolet (UV) treatment of smoothened PDMS replica, aluminum (Al) layer is deposited by thermal evaporation. Due to smoothened surface of PDMS replica, Al layer shows clear reflected image without perceptible lines, thereby functioning as a curved mirror. We expect that our curved mirror will be applicable to display and imaging devices.
Solution-processed polymer light-emitting diodes (PLEDs) have been widely investigated in display area due to their low-cost and large-scale fabrication. Generally, in order to pattern the device, the electrodes are deposited through a vacuum process such as sputtering or thermal evaporation. In terms of cost, inkjet printing is the most promising alternative to evaporation process because it allows low-material consumption as well as free patterning of the electrodes. However, direct inkjet-printing on the organic layers induces solvent permeation, which causes severe damage to underlying layers. In addition, fine patterns are hard to be obtained because the surface treatment on the functional layers is limited. In this research, we report solution-processed PLEDs with inkjet-printed electrodes. In order to prevent solvent permeation and obtain fine patterns by inkjet printing, we print top electrode on surface-modified polydimethylsiloxane (PDMS) substrate and laminate it on the organic functional layers. A structure of our devices is ITO (anode) / PEDOT :PSS (HIL) / PDY-132 (EML) / PEI (interlayer) / ZnO (EIL) / Ag (cathode). The device with laminated Ag shows a turn-on voltage of 2.7 V at 1 cd/m2 and a current efficiency of 7.8 cd/A at 1000 cd/m2, while the device with evaporated Ag shows 2.4 V and 9.9 cd/A under the same condition. Based on our lamination process, all solution-processed PLEDs are fabricated by replacing ITO to inkjet-printed PEDOT :PSS. Furthermore, passive-matrix application is demonstrated showing the possibilities of all solution-processed display. Detailed fabrication process and experimental results will be discussed at the conference.
We fabricated all solution-processed inverted polymer light emitting diodes (PLEDs) where functional layers were spin-coated on patterned-ITO glass substrates and PEDOT:PSS anodes were deposited by a transfer process. The structure of our devices is ITO (cathode) / ZnO (EITL) / PEI (interlayer) / PDY-132 (EML) / PEDOT:PSS (HITL) / transferred conductive PEDOT:PSS (anode). Although many groups have studied all solution-processed PLEDs, top electrodes were typically fabricated by photolithography or adhesive tape, which hinders low-cost and large-area mass production. In order to fabricate top electrodes which will not damage underlying organic layers and can be implemented in a facile manner, we used the transfer process. PEDOT:PSS was selected as the top electrodes because it can be patterned by a printing process such as an inkjet printing technique, and then the patterned PEDOT:PSS electrodes can be easily transferred. We fabricated two types of inverted PLEDs which have an evaporated Al or a transferred PEDOT:PSS top electrode. The device with the evaporated Al showed a turn-on voltage of 2.6 V defined at 1 cd/m2 and a current efficiency of 10.2 cd/A at 1000 cd/m2 while the one with the transferred PEDOT:PSS showed a turn-on voltage of 2.7 V and a current efficiency of 8.2 cd/A at the same condition. Difference in sheet resistance of the top electrode and thus, charge balance change probably caused the performance variation. When the bottom cathodes are inkjet-printed, all solution-processed inverted PLEDs can be implemented, which will be also presented at conference.
Elastomeric mirror is one of the main components of systems that require tunable optical characteristics, and is being applied in various devices such as optical zoom camera, electrostatic actuator, and augmented/virtual reality (AR/VR) display. Generally, to fabricate an elastomeric mirror, a metal layer is deposited on an elastomer substrate by vacuum process such as thermal evaporation, e-beam evaporation, and sputtering. However, these processes can damage the elastomeric substrate, thereby degrading the quality of the mirror surface. The metal layer formed on the elastomeric substrate is also vulnerable to small deformation, which limits applications of elastomeric mirror. In this work, we report all-solution-processed elastomeric mirror film whose constituent layers were deposited sequentially by spin coating and dip coating method. The film consists of polydimethylsiloxane (PDMS) base, aluminum (Al) mirror, and PDMS encapsulation layer. As a material of mirror layer, we selected a ‘mirror ink’, which composed of Al powder, organic solvent, adhesive and mainly used for screen printing. We adjusted the dilution concentration of mirror ink to make it suitable for the solution process and controlling the roughness of the coated mirror layer. In addition, there was no damage to the mirror layer against deformation due to the presence of encapsulation layer, so it can be attachable well to the curved surface. As an example of application, we demonstrated a seamless display system by placing the elastomeric mirror between two curved panels. We expect that our elastomeric mirror will be applicable to various tunable optical systems.
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