Paper
29 January 2008 Narrowing of the homogeneous two-photon absorption line width in two-level dipolar system
Author Affiliations +
Abstract
We study narrowing of nonlinear two photon absorption line shape in system with non-zero permanent dipole moment difference between the ground- and excited state. The temperature-induced broadening of one photon absorption (1PA) and two photon absorption (2PA) line shapes is modeled by subjecting the resonance transition frequency to random fluctuations of varying amplitude and by solving numerically the corresponding two-level density matrix equation of motion. We show that under conditions, when 1PA and 2PA transitions are both far from saturation, the 2PA homogeneous line width may be as much as 25% narrower than the corresponding 1PA line width. This offers novel possibilities for reducing the temperature-induced dephasing in quantum computing, quantum memory and other applications based on coherent multi-photon interactions.
© (2008) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Aleks K. Rebane, Mikhail A. Drobizhev, and Nikolay S. Makarov "Narrowing of the homogeneous two-photon absorption line width in two-level dipolar system", Proc. SPIE 6903, Advanced Optical Concepts in Quantum Computing, Memory, and Communication, 690305 (29 January 2008); https://doi.org/10.1117/12.761400
Lens.org Logo
CITATIONS
Cited by 1 scholarly publication.
Advertisement
Advertisement
RIGHTS & PERMISSIONS
Get copyright permission  Get copyright permission on Copyright Marketplace
KEYWORDS
Absorption

Molecules

Terahertz radiation

Modulation

Solids

Complex systems

Oscillators

Back to Top