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Controlling the formation, size distribution and orientation of quantum wells (QWs) in layered hybrid perovskite (LHP) thin films is foundational to their optoelectronic device applications. These applications require exquisite control of energy and charge transport which tend to be highly anisotropic in low-dimensional phases in LHP thin films. Here, we combine a powerful suite of multimodal in situ characterizations to elucidate the precise solution-to-solid conversion of the sol into the LHP thin film. We identify, for the first time, the presence of oriented colloidal transient nanostructures during spin coating well before the onset of crystallization of phases.
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Kasra Darabi, Dovletgeldi Seyitliyev, Boyu Guo, Fazel Bateni, Tonghui Wang, Masoud Ghasemi, Laine Taussig, Milad Abolhasani, Kenan Gundogdu, Aram Amassian, "Colloidal nanostructures control the formation and orientation of quantum wells in layered hybrid perovskites (Conference Presentation)," Proc. SPIE PC12208, Organic and Hybrid Light Emitting Materials and Devices XXVI, PC122080C (3 October 2022); https://doi.org/10.1117/12.2633675