We present a versatile characterisation of liquid crystal devices, including those integrated with organic photovoltaics. Photovoltaic thin film serves as an alignment layer and also generates an electric field under illumination that reorients liquid crystals for self-activated or autonomous operation. Apart polar alignment angle, anchoring energy, thickness uniformity, the photovoltaic properties, such as the photovoltage generated and photoconductivity, are captured and the map of the spatial changes of the parameters can be created. The method is applicable to other liquid crystal systems, such as doped liquid crystals and optically thin cells, with phase lag as small as π.
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