We have fabricated a spin photovoltaic device composed of a vertical spin-valve based on hybrid organic–inorganic perovskite as a spacer layer, of which resistance may be tuned by external light illumination. The magnetoconductivity of this device may be tuned from zero to reach exceptionally high values of 100 k% by controlling the illumination intensity close to the open circuit voltage. In addition, the device photocurrent can be also turned by sweeping the external magnetic field when the effects of the light intensity and applied bias voltage are judicially balanced.
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